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赵恺副教授课题组在Organic Letters期刊上发表研究论文
阅读次数: 添加时间:2020/11/30 发布:

Visible-Light-Induced Regio- & Stereoselective C(sp2)–H Trifluoroethylation of Enamides with 2,2,2-Trifluoroethyl Iodide

Kai Zhao,*,1 Ze-Yu Zhang,1,# Xian-Lu Cui,1,#Ying-Xue Wang,1# Xian-Dan Wu,1 Wei-Ming Li,1 Jia-Xu Wu,1 Li-Li Zhao,*,1 Jing-Yu Guo*,1 and Teck-Peng Loh,*,1,2

1Institute of Advanced Synthesis, School of Chemistry and Molecular Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing Tech University, Nanjing 211816, China.

2Division of Chemistry and Biological Chemistry, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore.

#These authors contributed equally.

Abstract: A photoredox-catalyzed regio- and stereoselective trifluoroethylation reaction of enamides using commercially available 2,2,2-trifluoroethyl iodide as trifluoroethylating agents has been developed, furnishing geometrically-defined and synthetically and physiochemically pivotal β-trifluoroethylated enamides bearing a diverse range of functional groups.

Org. Lett. 2020, 22, 9029. (2019年影响因子: 6.091).

论文链接:https://pubs.acs.org/doi/10.1021/acs.orglett.0c03418





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